Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe3O4/zeolite-NaY in methylene blue degradation

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Dinia Astira, Romario Abdullah, Utari Zulfiani, Dety Oktavia Sulistiono, Zeni Rahmawati, Triyanda Gunawan, Mohd Hafiz Dzarfan Othman, Muhammad Hasan, Ratna Ediati, Hamzah Fansuri

2024 Case Studies in Chemical and Environmental Engineering Vol. 10 Article Cited by 6 SDG 12SDG 17 Quartile

Abstract

A composite catalyst was developed to degrade methylene blue (MB) via the Fenton reaction from Fe3O4 and H2O2 with zeolite-NaY as magnetite support to reduce agglomeration. Hydrothermal and co-precipitation approaches were used to synthesize the composite. The co-precipitation method here was proven to be more suitable to produce the composite. Under optimal conditions, all composite catalysts achieved a remarkable MB reduction (more than 90 %) as confirmed through TLC analysis and UV–Vis spectra. Notably, based on linear regression, FeZ-A maintained over 60 % activity after 15 uses, while FeZ-2 showed the least Fe ion leaching. This demonstrated the effectiveness and stability of the developed catalysts. © 2024 The Authors

Affiliations

Departement of Chemistry, Faculty of Science and Data Analytics, Institut Teknologi Sepuluh Nopember, Sukolilo, Surabaya, 60111, Indonesia; Automotive Engineering, Engineering Department, Politeknik Negeri Jember, Jember, 68101, Indonesia; Advanced Membrane Technology Research Centre (AMTEC), Universiti Teknologi Malaysia, Skudai, Johor Bahru, 81310, Malaysia; Department of Chemistry Education, Faculty of Teacher Training and Education, Universitas Syiah Kuala, Darussalam, Banda Aceh, 23111, Indonesia

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